Long-Range Plasmon-Assisted Energy Transfer between Fluorescent Emitters.

نویسندگان

  • D Bouchet
  • D Cao
  • R Carminati
  • Y De Wilde
  • V Krachmalnicoff
چکیده

We demonstrate plasmon-assisted energy transfer between fluorophores located at distances up to 7  μm on the top of a thin silver film. Thanks to the strong confinement and large propagation length of surface plasmon polaritons, the range of the energy transfer is almost 2 orders of magnitude larger than the values reported in the literature so far. The parameters driving the energy transfer range are thoroughly characterized and are in very good agreement with theoretically expected values.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Observation of selective plasmon-exciton coupling in nonradiative energy transfer: donor-selective versus acceptor-selective plexcitons.

We report selectively plasmon-mediated nonradiative energy transfer between quantum dot (QD) emitters interacting with each other via Förster-type resonance energy transfer (FRET) under controlled plasmon coupling either to only the donor QDs (i.e., donor-selective) or to only the acceptor QDs (i.e., acceptor-selective). Using layer-by-layer assembled colloidal QD nanocrystal solids with metal ...

متن کامل

Control of plasmon emission and dynamics at the transition from classical to quantum coupling.

With nanosecond radiative lifetimes, quenching dominates over enhancement for conventional fluorescence emitters near metal interfaces. We explore the fundamentally distinct behavior of photoluminescence (PL) with few-femtosecond radiative lifetimes of a coupled plasmonic emitter. Controlling the emitter-surface distance with subnanometer precision by combining atomic force and scanning tunneli...

متن کامل

Excitonics of semiconductor quantum dots and wires for lighting and displays

R EV EW A R IC LE Abstract In the past two decades, semiconductor quantum dots and wires have developed into new, promising classes of materials for next-generation lighting and display systems due to their superior optical properties. In particular, exciton–exciton interactions through nonradiative energy transfer in hybrid systems of these quantum-confined structures have enabled exciting pos...

متن کامل

Exciton mobility and trapping in a MALDI matrix.

Energy transfer (ET) from excited matrix to fluorescent traps is used to probe the mobility of excitations in the matrix-assisted laser desorption/ionization (MALDI) matrix material 2,5-dihydroxybenzoic acid. The dependence of host and guest fluorescence on excitation density (laser intensity) and trap concentration gives clear evidence for long-range energy transport in this matrix. This concl...

متن کامل

Spectral Selectivity of Plasmonic Interactions between Individual Up-Converting Nanocrystals and Spherical Gold Nanoparticles

We experimentally demonstrate strong spectral selectivity of plasmonic interaction that occurs between α-NaYF₄:Er3+/Yb3+ nanocrystals, which feature two emission bands, and spherical gold nanoparticles, with plasmon frequency resonant with one of the emission bands. Spatially-resolved luminescence intensity maps acquired for individual nanocrystals, together with microsecond luminescence lifeti...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Physical review letters

دوره 116 3  شماره 

صفحات  -

تاریخ انتشار 2016